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Meeting 2025 TMS Annual Meeting & Exhibition
Symposium Characterization of Materials through High Resolution Coherent Imaging
Presentation Title Operando and Linear Dichroic Ptychographic Spectro-Tomography of Heterogenous Catalysts
Author(s) Johannes Ihli, Zirui Gao , Andreas Apseros Andreas, Appel Christian, Tomas Aidukas, Ana Diaz, Valerio Scagnoli, Andreas Menzel, Manuel Guizar Sicairos, Claire Donnelly , Jeroen van Bokhoven, Mirko Holler
On-Site Speaker (Planned) Johannes Ihli
Abstract Scope Heterogeneous catalysts drive numerous industrial processes, including chemical production, energy conversion, and environmental protection. Enhancing their efficiency and durability necessitates a deep understanding of the intricate relationships between their complex 3D structure, chemical makeup and performance. Bulk and or ambient-temperature characterization often fails to capture the complex nature of these catalysts under real operational conditions, creating a significant barrier to optimizing their design and functionality. Here, we present recent advances in the acquisition and analysis of (Operando) and Linear Dichroic Ptychographic Spectro-Tomography as a tool to facilitate a 3D compositional, chemical and or microstructural characterization of Heterogeneous Catalysts in their use-geometry under operational conditions. Presented are three studies ranging from model-supported catalysts to industrial in-use catalysts. Catalysts were examined at a spatial resolution of 20 nm at up to 800°C under contrasting atmospheres.
Proceedings Inclusion? Planned:
Keywords Characterization, Energy Conversion and Storage, Ceramics

OTHER PAPERS PLANNED FOR THIS SYMPOSIUM

AI-Driven Workflow for Autonomous High-Resolution Scanning X-Ray Microscopy
Bragg Coherent Diffractive Imaging With Twisted X-Rays
Characterization of Crystalline Materials at the Atomic Scale with X-Ray Bragg Coherent Diffraction Imaging
Coherent x-Ray Diffraction Imaging Dedicated Beamlines at PLS-II and Korea-4GSR
Direct Reciprocal Space Detection of Microelectronic Defects Using Coherent X-Ray Diffraction and Unsupervised Machine Learning
Enhanced Mineral Characterization With 3D X-Ray CT and AI-Driven Imaging
Explanation of the High-Dielectric Constant of BaTiO3 Used in Multilayer Capacitors
High-Resolution X-Ray Imaging of Integrated Circuits
High Bandwidth Scanning X-Ray Microscopy
In-Situ/Operando Bragg Coherent X-Ray Diffraction Imaging for Catalysis Studies
ML-Guided Non-Destructive 3D Metrology of Functioning Devices With an X-Ray Laser
Nanoholotomography With Coded Apertures for Efficient Dynamic Imaging of Nanomaterials
Operando and Linear Dichroic Ptychographic Spectro-Tomography of Heterogenous Catalysts
Origin of Structural Degradation in Layered Oxide Cathode for Li-Ion Batteries
Physics-Informed Self-Supervised Learning of Structural Morphology Imaged by Scanning X-Ray Diffraction Microscopy
Probing Cryogenic Strain Evolution in SrTiO3 Using Multi-Reflection Bragg Coherent Diffraction Imaging
Rapid Reconstruction of the Full Strain Tensor via Coupled Phase Retrieval With Multipeak Bragg Coherent Diffraction Imaging
Real-Time Imaging of Subsurface Dislocation Dynamics
Simultaneous Reciprocal and Real Space X-Ray Imaging for Hierarchical Characterization of 3D Nano-Architected Metamaterials
Single-Exposure Elemental Differentiation and Texture-Sensitive Phase-Retrieval Imaging with a Neutron-Counting Microchannel-Plate Detector
Single-Shot X-Ray Imaging of Density in Laser Shocked Materials for Fusion Energy Studies
Synchrotron Ptychographic X-Ray Computed Tomography (PXCT) to Study Micro-Fabricated Fully Hybrid 3D Metal-Ceramic Metamaterials
Three-Dimensional Hard X-Ray Ptychographic Reflectometry Imaging on Extended Mesoscopic Surface Structures

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