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Meeting 2025 TMS Annual Meeting & Exhibition
Symposium Characterization of Materials through High Resolution Coherent Imaging
Presentation Title Probing Cryogenic Strain Evolution in SrTiO3 Using Multi-Reflection Bragg Coherent Diffraction Imaging
Author(s) David Yang, Sung Soo Ha, Sung Wook Choi, Jialun Liu, Daniel Treuherz, Longlong Wu, Ana F Suzana, Gareth Nisbet, Dan Porter, Hyunjung Kim, Ian K Robinson
On-Site Speaker (Planned) David Yang
Abstract Scope Strontium titanate (STO) is a complex oxide perovskite relevant for capacitors, semiconductors, and superconductors, exhibiting significant physics phenomena due to its mixed ionic and covalent properties. STO undergoes a well-known cubic-to-tetragonal (antiferrodistortive) phase transition at 105 K, which is close to a quantum critical point related to superconductivity. However, the size dependence of this phase transition is not widely reported. Here we explore the phase transition in STO microcrystals using in operando multi-reflection Bragg coherent diffraction imaging (BCDI), to examine 3D strain tensor evolution at cryogenic temperatures. Heatmap analysis of 3D tensor components capture structural modes, and we note voids of missing electron density associated with SrCO3 impurities. Quantitative changes in the strain fields surrounding 1/2<011> type dislocations are observed as a function of radial position and increase in magnitude as a function of decreasing temperature. Understanding these low-temperature structural changes is crucial for developing next-generation electronic devices.
Proceedings Inclusion? Planned:
Keywords Other, Characterization, Other

OTHER PAPERS PLANNED FOR THIS SYMPOSIUM

AI-Driven Workflow for Autonomous High-Resolution Scanning X-Ray Microscopy
Bragg Coherent Diffractive Imaging With Twisted X-Rays
Characterization of Crystalline Materials at the Atomic Scale with X-Ray Bragg Coherent Diffraction Imaging
Coherent x-Ray Diffraction Imaging Dedicated Beamlines at PLS-II and Korea-4GSR
Direct Reciprocal Space Detection of Microelectronic Defects Using Coherent X-Ray Diffraction and Unsupervised Machine Learning
Enhanced Mineral Characterization With 3D X-Ray CT and AI-Driven Imaging
Explanation of the High-Dielectric Constant of BaTiO3 Used in Multilayer Capacitors
High-Resolution X-Ray Imaging of Integrated Circuits
High Bandwidth Scanning X-Ray Microscopy
In-Situ/Operando Bragg Coherent X-Ray Diffraction Imaging for Catalysis Studies
ML-Guided Non-Destructive 3D Metrology of Functioning Devices With an X-Ray Laser
Nanoholotomography With Coded Apertures for Efficient Dynamic Imaging of Nanomaterials
Operando and Linear Dichroic Ptychographic Spectro-Tomography of Heterogenous Catalysts
Origin of Structural Degradation in Layered Oxide Cathode for Li-Ion Batteries
Physics-Informed Self-Supervised Learning of Structural Morphology Imaged by Scanning X-Ray Diffraction Microscopy
Probing Cryogenic Strain Evolution in SrTiO3 Using Multi-Reflection Bragg Coherent Diffraction Imaging
Rapid Reconstruction of the Full Strain Tensor via Coupled Phase Retrieval With Multipeak Bragg Coherent Diffraction Imaging
Real-Time Imaging of Subsurface Dislocation Dynamics
Simultaneous Reciprocal and Real Space X-Ray Imaging for Hierarchical Characterization of 3D Nano-Architected Metamaterials
Single-Exposure Elemental Differentiation and Texture-Sensitive Phase-Retrieval Imaging with a Neutron-Counting Microchannel-Plate Detector
Single-Shot X-Ray Imaging of Density in Laser Shocked Materials for Fusion Energy Studies
Synchrotron Ptychographic X-Ray Computed Tomography (PXCT) to Study Micro-Fabricated Fully Hybrid 3D Metal-Ceramic Metamaterials
Three-Dimensional Hard X-Ray Ptychographic Reflectometry Imaging on Extended Mesoscopic Surface Structures

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