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Meeting 2025 TMS Annual Meeting & Exhibition
Symposium Thin Films and Coatings: Properties, Processing and Applications
Presentation Title Exploring the Mechano-Chemical Response of Pt-based Thin Films using Automated High Throughput Testing
Author(s) Tomas F. Babuska, Justin M Hall, Joyce O Custer, Sadhvikas J Addamane, David P Adams, Brad P Boyce, Frank W DelRio, John F Curry
On-Site Speaker (Planned) Tomas F. Babuska
Abstract Scope Thermally stable Pt-based nanocrystalline alloy coatings are promising candidates for electrical contact materials with improved friction/wear. Pt-Au coatings have been shown to form super-lubricious carbon-based surface films (µ < 0.05) from adventitious carbon when operated in inert environments. Pt-rich coatings (> 90 at. % Pt) have been studied showing relationships between composition and hardness on the mechano-chemical response. In this work, Pt-Au combinatorial libraries made via physical vapor deposition are assessed using a novel semi-autonomous friction/wear testing apparatus (tribometer). We highlight the mechano-chemical response of 448 Pt-Au coatings spanning ~0-100 at. % Pt and correlations with hardness, composition, and density. This study demonstrates how ~1000 unique tests can be performed a few days allowing for the generation of large multi-modal experimental data sets suitable for machine learning models that can aide in the discovery of novel material solutions. SNL is managed and operated by NTESS under DOE NNSA contract DE-NA0003525.
Proceedings Inclusion? Planned:
Keywords Thin Films and Interfaces, Surface Modification and Coatings, Mechanical Properties

OTHER PAPERS PLANNED FOR THIS SYMPOSIUM

2D Simulation of Silicon Solar Cells
A new electrochemical sensor for lithium hexafluorophosphate detection
A Plasma Diagnostic Based Approach to Accelerate the Process Development of High Performance MoS2
A Review of Coating Processes for Engineering Surfaces in Harsh Environments
Active Learning and Transfer Learning for Rapid Targeted Synthesis of Compositionally Complex Thin Film Alloys
Carbon Nanotube Coating for Tribological and Thermal Applications
Charge redistribution around threading dislocations in III-nitride epilayers
Deposition and corrosion resistivity of a novel multilayer PEO-HEA coating on Mg alloy
Design of interpenetrating composite coatings for extreme environments
Developing Functional Metrics to Predict Performance & Aging Properties of MoS2 Thin Films
Doping/Alloying Enabled Tunable Optical Properties of Epitaxial β-Ga2O3 Thin Films
Effect of Deep Cryogenic Treatment on the Structure and Properties of Ni-Co-Cr Alloy Coating
Effect of Sol-Gel-Based Dielectric Coatings on Silicon Radiative Properties
Effect of Thermal Bi-metal coating on the transformation temperatures and thermal hysteresis of NiTi SMA / Flexinol® wires.
Effects of Environmental Species on Tribological Properties of MoS2: Using Simulations to Interpret Experimental Observations
Electro-mechanical behavior of indium tin oxide thin films deposited on flexible substrates
Enhanced Condensation Performance of High-Power Vapor Chamber by Electrodeposition and Surface Modification
Enhancing Boiling Heat Transfer Performance of Superhydrophilic Cu Films with Electrodeposited Dendritic Structure
Exploring the Mechano-Chemical Response of Pt-based Thin Films using Automated High Throughput Testing
Exploring Thin Films for Promising Biomedical Applications: An Overview
High-throughput exploration of ultrastrong nanocrystalline CoCr alloys
Hydrophobic Behaviour of Polyurethane based Metal Oxide Composite Coating for the Protection of Ancient Artefacts and Monuments
Improving the Bonding Conditions Between Metal and Polymer for Sandwich Sheet Materials
Influence of HFCVD Diamond Coatings on the Friction and Adhesion in Aluminum and Magnesium Extrusion
Laser-induced Oxidation Phase Diagrams: Opportunities for High Throughput Thin Film Optimization
Linking Pt-Au Alloy Composition and Surface Mechanocatalytic Activity
Low-cost chemical deposition techniques of various thin films onto various substrates with enhanced properties
Magnetic nanocomposites for Flexible Magneto-Electronics
Material and Device Engineering for Multi Kilo Volt Class Vertical Ga2O3 Devices
Microstructural characterization and mechanical behavior of Mg-Ti Alloys Fabricated by Physical Vapor Deposition
MOF-based self-healing coating material with triple distinct and efficient healing bond for preventing fat, oil and grease deposition and corrosion in sewer system
Multilayer optical filters for spectral analysis of trace elements in aluminum
Optical and structural characterization of highly doped nanocrystals based on group IV semiconductors by for plasmonic applications
Plasma-assisted surface treatment and coating deposition on AZ91D and AM60 Mg Alloys for Corrosion Protection
Pseudocapacitive Behaviour of Zn-TiO2-SnO2 Nano-Composite Coatings
Reactive Multilayer Induced Self-Healing in Thin Films – The Importance of Diffusion Barriers
Recent progress of antifogging coating on glasses/lenses: a short review
Role of Surface Chemistry on the Growth of Plasma Polymers Thin Films
Role of the Si content in the LME susceptibility of the Zn-coated QP980 advanced high strength steel
Spectro-microscopy of the local chemistry and structure of thin films
Strain Effects on Adatom Diffusion, Island Nucleation and Monolayer Growth on Metal and Oxide Surfaces
Synthesis and heat treatment conditions in Zn1−xFexO nanoparticles
Synthesis of phase change microcapsules for thermal management film of electronic devices using pickering emulsion.
Synthesis, microstructure, and interfacial/surface properties of TeO2-core/TiO2-shell nanowires
Systematic control of crystallization temperature of amorphous NiTi films using seed crystals
Thermal Measurements at the Nano-scale: Theory, Reality, and Examples
Thermal Stability and Mechanical Properties of μ-Phase Composition W-Fe-Ni-Mo Multi-Principal Element Alloy Film
Transition Metal Dependency on the Hardness of Sputter Deposited Metal Carbide Thin Films
Tribosintering of nanocrystals – Manufacturing wear-resistant TiO2 coatings at ambient temperature
Ultra-fast Synthesis of Superhard Borides of W, Re, and WRe (20%Re) Alloys Using Electrochemical Boriding

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